dorsal/arxiv
View SchemaDissociation spectrum of H$_2^+$ from a short, intense infrared laser pulse: vibration structure and focal volume effects
| Authors | Liang-You Peng, I D Williams, J F McCann |
|---|---|
| Categories | |
| ArXiv ID | physics/0412075 |
| URL | https://arxiv.org/abs/physics/0412075 |
| DOI | 10.1088/0953-4075/38/11/014 |
| Journal | J. Phys. B: At. Mol. Opt. Phys. 38 (2005) 1727-1743 |
Abstract
The dissociation spectrum of the hydrogen molecular ion by short intense pulses of infrared light is calculated. The time-dependent Schr\"odinger equation is discretized and integrated in position and momentum space. For few-cycle pulses one can resolve vibrational structure that commonly arises in the experimental preparation of the molecular ion from the neutral molecule. We calculate the corresponding energy spectrum and analyze the dependence on the pulse time-delay, pulse length, and intensity of the laser for $\lambda \sim 790$nm. We conclude that the proton spectrum is a both a sensitive probe of the vibrational dynamics and the laser pulse. Finally we compare our results with recent measurements of the proton spectrum for 55 fs pulses using a Ti:Sapphire laser ($\lambda \sim 790 $nm). Integrating over the laser focal volume, for the intensity $I \sim 3 \times 10^{15}$W cm$^{-2}$, we find our results are in excellent agreement with these experiments.
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"abstract": "The dissociation spectrum of the hydrogen molecular ion by short intense\npulses of infrared light is calculated. The time-dependent Schr\\\"odinger\nequation is discretized and integrated in position and momentum space. For\nfew-cycle pulses one can resolve vibrational structure that commonly arises in\nthe experimental preparation of the molecular ion from the neutral molecule. We\ncalculate the corresponding energy spectrum and analyze the dependence on the\npulse time-delay, pulse length, and intensity of the laser for $\\lambda \\sim\n790$nm. We conclude that the proton spectrum is a both a sensitive probe of the\nvibrational dynamics and the laser pulse. Finally we compare our results with\nrecent measurements of the proton spectrum for 55 fs pulses using a Ti:Sapphire\nlaser ($\\lambda \\sim 790 $nm). Integrating over the laser focal volume, for the\nintensity $I \\sim 3 \\times 10^{15}$W cm$^{-2}$, we find our results are in\nexcellent agreement with these experiments.",
"arxiv_id": "physics/0412075",
"authors": [
"Liang-You Peng",
"I D Williams",
"J F McCann"
],
"categories": [
"physics.atom-ph",
"physics.chem-ph",
"physics.comp-ph"
],
"doi": "10.1088/0953-4075/38/11/014",
"journal_ref": "J. Phys. B: At. Mol. Opt. Phys. 38 (2005) 1727-1743",
"title": "Dissociation spectrum of H$_2^+$ from a short, intense infrared laser pulse: vibration structure and focal volume effects",
"url": "https://arxiv.org/abs/physics/0412075"
},
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