dorsal/arxiv
View SchemaSingle-Shot Two Dimensional Time Resolved Coherent Anti Stokes Raman Scattering
| Authors | Yuri Paskover, I. Sh. Averbukh, Yehiam Prior |
|---|---|
| Categories | |
| ArXiv ID | physics/0612057 |
| URL | https://arxiv.org/abs/physics/0612057 |
| DOI | 10.1364/OE.15.001700 |
Abstract
Single-shot time resolved Coherent Anti-Stokes Raman Scattering (CARS) is presented as a viable method for fast measurements of molecular spectra. The method is based on the short spatial extension of femtosecond pulses and maps time delays between pulses onto the region of intersection between broad beams. The image of the emitted CARS signal contains full temporal information on the field-free molecular dynamics, from which spectral information is extracted. The method is demonstrated on liquid samples of CHBr3 and CHCl3 and the Raman spectrum of the low-lying vibrational states of these molecules is measured.
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"abstract": "Single-shot time resolved Coherent Anti-Stokes Raman Scattering (CARS) is\npresented as a viable method for fast measurements of molecular spectra. The\nmethod is based on the short spatial extension of femtosecond pulses and maps\ntime delays between pulses onto the region of intersection between broad beams.\nThe image of the emitted CARS signal contains full temporal information on the\nfield-free molecular dynamics, from which spectral information is extracted.\nThe method is demonstrated on liquid samples of CHBr3 and CHCl3 and the Raman\nspectrum of the low-lying vibrational states of these molecules is measured.",
"arxiv_id": "physics/0612057",
"authors": [
"Yuri Paskover",
"I. Sh. Averbukh",
"Yehiam Prior"
],
"categories": [
"physics.optics"
],
"doi": "10.1364/OE.15.001700",
"title": "Single-Shot Two Dimensional Time Resolved Coherent Anti Stokes Raman Scattering",
"url": "https://arxiv.org/abs/physics/0612057"
},
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