dorsal/arxiv
View SchemaWhat can be learned about molecular reorientation from single molecule polarization microscopy?
| Authors | M. F. Gelin, D. S. Kosov |
|---|---|
| Categories | |
| ArXiv ID | physics/0611110 |
| URL | https://arxiv.org/abs/physics/0611110 |
| DOI | 10.1063/1.2227395 |
| Journal | J. Chem. Phys. 125, 054708 (2006) |
Abstract
We have developed a general approach for the calculation of the single molecule polarization correlation function C(t), which delivers a correlation of the emission dichroisms at time 0 and t. The approach is model independent and valid for general asymmetric top molecules. The key dynamic quantities of our analysis are the even-rank orientational correlation functions, the weighted sum of which yields C(t). We have demonstrated that the use of non-orthogonal schemes for the detection of the single molecule polarization responses makes it possible to manipulate the weighting coefficients in the expansion of C(t). Thus valuable information about the orientational correlation functions of the rank higher than second can be extracted from C(t).
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"abstract": "We have developed a general approach for the calculation of the single\nmolecule polarization correlation function C(t), which delivers a correlation\nof the emission dichroisms at time 0 and t. The approach is model independent\nand valid for general asymmetric top molecules. The key dynamic quantities of\nour analysis are the even-rank orientational correlation functions, the\nweighted sum of which yields C(t). We have demonstrated that the use of\nnon-orthogonal schemes for the detection of the single molecule polarization\nresponses makes it possible to manipulate the weighting coefficients in the\nexpansion of C(t). Thus valuable information about the orientational\ncorrelation functions of the rank higher than second can be extracted from\nC(t).",
"arxiv_id": "physics/0611110",
"authors": [
"M. F. Gelin",
"D. S. Kosov"
],
"categories": [
"physics.chem-ph",
"physics.optics"
],
"doi": "10.1063/1.2227395",
"journal_ref": "J. Chem. Phys. 125, 054708 (2006)",
"title": "What can be learned about molecular reorientation from single molecule polarization microscopy?",
"url": "https://arxiv.org/abs/physics/0611110"
},
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