{
  "annotation_id": "4fdb04d1-544f-4245-ac89-8573a545121b",
  "date_created": "2026-03-02T18:01:55.595000Z",
  "date_modified": "2026-03-02T18:01:55.595000Z",
  "file_hash": "671cf36a7a16d3fa5b500b7616f24b6311edac9de3ce938337d9de5169d3d2e4",
  "private": false,
  "record": {
    "abstract": "A spectroscopic application of the atom laser is suggested. The spectroscopy\ntermed 2PACC employs the coherent properties of matter-waves from a two pulse\natom laser. These waves are employed to control a gas-surface chemical\nrecombination reaction. The method is demonstrated for an Eley-Rideal reaction\nof a hydrogen or alkali atom-laser pulse where the surface target is an\nadsorbed hydrogen atom. The reaction yields either a hydrogen or alkali hydride\nmolecule. The desorbed gas phase molecular yield and its internal state is\nshown to be controlled by the time and phase delay between two atom-laser\npulses. The calculation is based on solving the time-dependent Schrodinger\nequation in a diabatic framework. The probability of desorption which is the\npredicted 2PACC signal has been calculated as a function of the pulse\nparameters.",
    "arxiv_id": "quant-ph/0301134",
    "authors": [
      "Solvejg Jorgensen",
      "Ronnie Kosloff"
    ],
    "categories": [
      "quant-ph",
      "physics.chem-ph"
    ],
    "doi": "10.1063/1.1576383",
    "journal_ref": "Journal of Chemical Physics, 119:149, (2003)",
    "title": "Two-Pulse Atomic Coherent Control (2PACC) Spectroscopy of Eley-Rideal   Reactions. An Application of an Atom Laser",
    "url": "https://arxiv.org/abs/quant-ph/0301134"
  },
  "schema_id": "dorsal/arxiv",
  "source": {
    "execution_id": "54031213-69cd-4c45-8cb6-d0f9eb5b92df",
    "id": "arXiv Dataset IDs",
    "type": "Model",
    "variant": "snapshot-2026-03-01",
    "version": "0.1.0"
  },
  "user_id": 1000002
}