{
  "annotation_id": "4ed60515-6109-4bda-ba20-20457a1429f1",
  "date_created": "2026-03-02T18:02:30.962000Z",
  "date_modified": "2026-03-02T18:02:30.962000Z",
  "file_hash": "14b27c0c8f880609e717f4906d151d60e37f91e1f88199ff293a7b062e0f59f0",
  "private": false,
  "record": {
    "abstract": "We present a general and highly efficient scheme for performing narrow-band\nRaman transitions between molecular vibrational levels using a coherent train\nof weak pump-dump pairs of shaped ultrashort pulses. The use of weak pulses\npermits an analytic description within the framework of coherent control in the\nperturbative regime, while coherent accumulation of many pulse pairs enables\nnear unity transfer efficiency with a high spectral selectivity, thus forming a\npowerful combination of pump-dump control schemes and the precision of the\nfrequency comb. The concept is presented analytically and its feasibility and\nrobustness are verified by simulations of dynamics in Rb$_2$. We consider\napplication of this concept to the formation of stable, deeply bound, ultracold\nmolecules.",
    "arxiv_id": "quant-ph/0609008",
    "authors": [
      "Avi Pe\u0027er",
      "Evgeny A. Shapiro",
      "Matthew C. Stowe",
      "Moshe Shapiro",
      "Jun Ye"
    ],
    "categories": [
      "quant-ph",
      "physics.atm-clus",
      "physics.atom-ph",
      "physics.optics"
    ],
    "doi": "10.1103/PhysRevLett.98.113004",
    "journal_ref": "Phys. Rev. Lett. 98, 113004 (2007)",
    "title": "Precise Control of Molecular Dynamics with a Femtosecond Frequency Comb   - A Weak Field Route to Strong Field Coherent Control",
    "url": "https://arxiv.org/abs/quant-ph/0609008"
  },
  "schema_id": "dorsal/arxiv",
  "source": {
    "execution_id": "e6935c56-601b-4da0-9a95-f3c3e6a9e765",
    "id": "arXiv Dataset IDs",
    "type": "Model",
    "variant": "snapshot-2026-03-01",
    "version": "0.1.0"
  },
  "user_id": 1000002
}