dorsal/arxiv
View SchemaSpectroscopic study of unique line broadening and inversion in low-pressure microwave generated water plasmas
| Authors | R. L. Mills, P. C. Ray, R. M. Mayo, M. Nansteel, B. Dhandapani, Jonathan Phillips |
|---|---|
| Categories | |
| ArXiv ID | physics/0401103 |
| URL | https://arxiv.org/abs/physics/0401103 |
| DOI | 10.1017/S0022377805003703 |
Abstract
It was demonstrated that low pressure (~0.2 Torr) water vapor plasmas generated in a 10 mm inner diameter quartz tube with an Evenson microwave cavity show at least two features which are not explained by conventional plasma models. First, significant (> 0.25 nm) hydrogen Balmer_ line broadening, of constant width, up to 5 cm from the microwave coupler was recorded. Only hydrogen, and not oxygen, showed significant line broadening. This feature, observed previously in hydrogen-containing mixed gas plasmas generated with high voltage dc and rf discharges was explained by some researchers to result from acceleration of hydrogen ions near the cathode. This explanation cannot apply to the line broadening observed in the (electrodeless) microwave plasmas generated in this work, particularly at distances as great as 5 cm from the microwave coupler. Second, inversion of the line intensities of both the Lyman and Balmer series, again, at distances up to 5 cm from the coupler, were observed. The line inversion suggests the existence of a hitherto unknown source of pumping of the optical power in plasmas. Finally, it is notable that other aspects of the plasma including the OH* rotational temperature and low electron concentrations are quite typical of plasmas of this type.
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"abstract": "It was demonstrated that low pressure (~0.2 Torr) water vapor plasmas\ngenerated in a 10 mm inner diameter quartz tube with an Evenson microwave\ncavity show at least two features which are not explained by conventional\nplasma models. First, significant (\u003e 0.25 nm) hydrogen Balmer_ line broadening,\nof constant width, up to 5 cm from the microwave coupler was recorded. Only\nhydrogen, and not oxygen, showed significant line broadening. This feature,\nobserved previously in hydrogen-containing mixed gas plasmas generated with\nhigh voltage dc and rf discharges was explained by some researchers to result\nfrom acceleration of hydrogen ions near the cathode. This explanation cannot\napply to the line broadening observed in the (electrodeless) microwave plasmas\ngenerated in this work, particularly at distances as great as 5 cm from the\nmicrowave coupler. Second, inversion of the line intensities of both the Lyman\nand Balmer series, again, at distances up to 5 cm from the coupler, were\nobserved. The line inversion suggests the existence of a hitherto unknown\nsource of pumping of the optical power in plasmas. Finally, it is notable that\nother aspects of the plasma including the OH* rotational temperature and low\nelectron concentrations are quite typical of plasmas of this type.",
"arxiv_id": "physics/0401103",
"authors": [
"R. L. Mills",
"P. C. Ray",
"R. M. Mayo",
"M. Nansteel",
"B. Dhandapani",
"Jonathan Phillips"
],
"categories": [
"physics.plasm-ph"
],
"doi": "10.1017/S0022377805003703",
"title": "Spectroscopic study of unique line broadening and inversion in low-pressure microwave generated water plasmas",
"url": "https://arxiv.org/abs/physics/0401103"
},
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